School of Earth Sciences - Research Publications

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    Dominant regions and drivers of the variability of the global land carbon sink across timescales
    Zhang, X ; Wang, Y-P ; Peng, S ; Rayner, PJ ; Ciais, P ; Silver, JD ; Piao, S ; Zhu, Z ; Lu, X ; Zheng, X (WILEY, 2018-09)
    Net biome productivity (NBP) dominates the observed large variation of atmospheric CO2 annual increase over the last five decades. However, the dominant regions controlling inter-annual to multi-decadal variability of global NBP are still controversial (semi-arid regions vs. temperate or tropical forests). By developing a theory for partitioning the variance of NBP into the contributions of net primary production (NPP) and heterotrophic respiration (Rh ) at different timescales, and using both observation-based atmospheric CO2 inversion product and the outputs of 10 process-based terrestrial ecosystem models forced by 110-year observational climate, we tried to reconcile the controversy by showing that semi-arid lands dominate the variability of global NBP at inter-annual (<10 years) and tropical forests dominate at multi-decadal scales (>30 years). Results further indicate that global NBP variability is dominated by the NPP component at inter-annual timescales, and is progressively controlled by Rh with increasing timescale. Multi-decadal NBP variations of tropical rainforests are modulated by the Pacific Decadal Oscillation (PDO) through its significant influences on both temperature and precipitation. This study calls for long-term observations for the decadal or longer fluctuations in carbon fluxes to gain insights on the future evolution of global NBP, particularly in the tropical forests that dominate the decadal variability of land carbon uptake and are more effective for climate mitigation.
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    Multi-species chemical data assimilation with the Danish Eulerian hemispheric model: system description and verification
    Silver, JD ; Christensen, JH ; Kahnert, M ; Robertson, L ; Rayner, PJ ; Brandt, J (SPRINGER, 2016-09)
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    A small climate-amplifying effect of climate-carbon cycle feedback
    Zhang, X ; Wang, Y-P ; Rayner, PJ ; Ciais, P ; Huang, K ; Luo, Y ; Piao, S ; Wang, Z ; Xia, J ; Zhao, W ; Zheng, X ; Tian, J ; Zhang, Y (NATURE PORTFOLIO, 2021-05-19)
    The climate-carbon cycle feedback is one of the most important climate-amplifying feedbacks of the Earth system, and is quantified as a function of carbon-concentration feedback parameter (β) and carbon-climate feedback parameter (γ). However, the global climate-amplifying effect from this feedback loop (determined by the gain factor, g) has not been quantified from observations. Here we apply a Fourier analysis-based carbon cycle feedback framework to the reconstructed records from 1850 to 2017 and 1000 to 1850 to estimate β and γ. We show that the β-feedback varies by less than 10% with an average of 3.22 ± 0.32 GtC ppm-1 for 1880-2017, whereas the γ-feedback increases from -33 ± 14 GtC K-1 on a decadal scale to -122 ± 60 GtC K-1 on a centennial scale for 1000-1850. Feedback analysis further reveals that the current amplification effect from the carbon cycle feedback is small (g is 0.01 ± 0.05), which is much lower than the estimates by the advanced Earth system models (g is 0.09 ± 0.04 for the historical period and is 0.15 ± 0.08 for the RCP8.5 scenario), implying that the future allowable CO2 emissions could be 9 ± 7% more. Therefore, our findings provide new insights about the strength of climate-carbon cycle feedback and about observational constraints on models for projecting future climate.
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    Evaluation of Regional Air Quality Models over Sydney, Australia: Part 2, Comparison of PM2.5 and Ozone
    Guerette, E-A ; Chang, LT-C ; Cope, ME ; Duc, HN ; Emmerson, KM ; Monk, K ; Rayner, PJ ; Scorgie, Y ; Silver, JD ; Simmons, J ; Trieu, T ; Utembe, SR ; Zhang, Y ; Paton-Walsh, C (MDPI, 2020-03)
    Accurate air quality modelling is an essential tool, both for strategic assessment (regulation development for emission controls) and for short-term forecasting (enabling warnings to be issued to protect vulnerable members of society when the pollution levels are predicted to be high). Model intercomparison studies are a valuable support to this work, being useful for identifying any issues with air quality models, and benchmarking their performance against international standards, thereby increasing confidence in their predictions. This paper presents the results of a comparison study of six chemical transport models which have been used to simulate short-term hourly to 24 hourly concentrations of fine particulate matter less than and equal to 2.5 µm in diameter (PM2.5) and ozone (O3) for Sydney, Australia. Model performance was evaluated by comparison to air quality measurements made at 16 locations for O3 and 5 locations for PM2.5, during three time periods that coincided with major atmospheric composition measurement campaigns in the region. These major campaigns included daytime measurements of PM2.5 composition, and so model performance for particulate sulfate (SO42−), nitrate (NO3−), ammonium (NH4+) and elemental carbon (EC) was evaluated at one site per modelling period. Domain-wide performance of the models for hourly O3 was good, with models meeting benchmark criteria and reproducing the observed O3 production regime (based on the O3/NOx indicator) at 80% or more of the sites. Nevertheless, model performance was worse at high (and low) O3 percentiles. Domain-wide model performance for 24 h average PM2.5 was more variable, with a general tendency for the models to under-predict PM2.5 concentrations during the summer and over-predict PM2.5 concentrations in the autumn. The modelling intercomparison exercise has led to improvements in the implementation of these models for Sydney and has increased confidence in their skill at reproducing observed atmospheric composition.
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    The shared socio-economic pathway (SSP) greenhouse gas concentrations and their extensions to 2500
    Meinshausen, M ; Nicholls, ZRJ ; Lewis, J ; Gidden, MJ ; Vogel, E ; Freund, M ; Beyerle, U ; Gessner, C ; Nauels, A ; Bauer, N ; Canadell, JG ; Daniel, JS ; John, A ; Krummel, PB ; Luderer, G ; Meinshausen, N ; Montzka, SA ; Rayner, PJ ; Reimann, S ; Smith, SJ ; van den Berg, M ; Velders, GJM ; Vollmer, MK ; Wang, RHJ (COPERNICUS GESELLSCHAFT MBH, 2020-08-13)
    Abstract. Anthropogenic increases in atmospheric greenhouse gas concentrations are the main driver of current and future climate change. The integrated assessment community has quantified anthropogenic emissions for the shared socio-economic pathway (SSP) scenarios, each of which represents a different future socio-economic projection and political environment. Here, we provide the greenhouse gas concentrations for these SSP scenarios – using the reduced-complexity climate–carbon-cycle model MAGICC7.0. We extend historical, observationally based concentration data with SSP concentration projections from 2015 to 2500 for 43 greenhouse gases with monthly and latitudinal resolution. CO2 concentrations by 2100 range from 393 to 1135 ppm for the lowest (SSP1-1.9) and highest (SSP5-8.5) emission scenarios, respectively. We also provide the concentration extensions beyond 2100 based on assumptions regarding the trajectories of fossil fuels and land use change emissions, net negative emissions, and the fraction of non-CO2 emissions. By 2150, CO2 concentrations in the lowest emission scenario are approximately 350 ppm and approximately plateau at that level until 2500, whereas the highest fossil-fuel-driven scenario projects CO2 concentrations of 1737 ppm and reaches concentrations beyond 2000 ppm by 2250. We estimate that the share of CO2 in the total radiative forcing contribution of all considered 43 long-lived greenhouse gases increases from 66 % for the present day to roughly 68 % to 85 % by the time of maximum forcing in the 21st century. For this estimation, we updated simple radiative forcing parameterizations that reflect the Oslo Line-By-Line model results. In comparison to the representative concentration pathways (RCPs), the five main SSPs (SSP1-1.9, SSP1-2.6, SSP2-4.5, SSP3-7.0, and SSP5-8.5) are more evenly spaced and extend to lower 2100 radiative forcing and temperatures. Performing two pairs of six-member historical ensembles with CESM1.2.2, we estimate the effect on surface air temperatures of applying latitudinally and seasonally resolved GHG concentrations. We find that the ensemble differences in the March–April–May (MAM) season provide a regional warming in higher northern latitudes of up to 0.4 K over the historical period, latitudinally averaged of about 0.1 K, which we estimate to be comparable to the upper bound (∼5 % level) of natural variability. In comparison to the comparatively straight line of the last 2000 years, the greenhouse gas concentrations since the onset of the industrial period and this studies' projections over the next 100 to 500 years unequivocally depict a “hockey-stick” upwards shape. The SSP concentration time series derived in this study provide a harmonized set of input assumptions for long-term climate science analysis; they also provide an indication of the wide set of futures that societal developments and policy implementations can lead to – ranging from multiple degrees of future warming on the one side to approximately 1.5 ∘C warming on the other.
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    The potential of Orbiting Carbon Observatory-2 data to reduce the uncertainties in CO2 surface fluxes over Australia using a variational assimilation scheme
    Villalobos, Y ; Rayner, P ; Thomas, S ; Silver, J (COPERNICUS GESELLSCHAFT MBH, 2020-07-21)
    This paper addresses the question of how much uncertainties in CO2 fluxes over Australia can be reduced by assimilation of total-column carbon dioxide retrievals from the Orbiting Carbon Observatory-2 (OCO-2) satellite instrument. We apply a four-dimensional variational data assimilation system, based around the Community Multiscale Air Quality (CMAQ) transport-dispersion model. We ran a series of observing system simulation experiments to estimate posterior error statistics of optimized monthly-mean CO2 fluxes in Australia. Our assimilations were run with a horizontal grid resolution of 81 km using OCO-2 data for 2015. Based on four representative months, we find that the integrated flux uncertainty for Australia is reduced from 0.52 to 0.13 Pg C yr−1. Uncertainty reductions of up to 90 % were found at grid-point resolution over productive ecosystems. Our sensitivity experiments show that the choice of the correlation structure in the prior error covariance plays a large role in distributing information from the observations. We also found that biases in the observations would significantly impact the inverted fluxes and could contaminate the final results of the inversion. Biases in prior fluxes are generally removed by the inversion system. Biases in the boundary conditions have a significant impact on retrieved fluxes, but this can be mitigated by including boundary conditions in our retrieved parameters. In general, results from our idealized experiments suggest that flux inversions at this unusually fine scale will yield useful information on the carbon cycle at continental and finer scales.
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    Data assimilation using an ensemble of models: a hierarchical approach
    Rayner, P (COPERNICUS GESELLSCHAFT MBH, 2020-03-27)
    Abstract. One characteristic of biogeochemical models is uncertainty about their formulation. Data assimilation should take this uncertainty into account. A common approach is to use an ensemble of models. We must assign probabilities not only to the parameters of the models but also to the models themselves. The method of hierarchical modelling allows us to calculate these probabilities. This paper describes the approach, develops the algebra for the most common case and then applies it to the Atmospheric Tracer Transport Model Intercomparison Project (TransCom). We see that the discrimination among models is unrealistically strong, due to optimistic assumptions inherent in the underlying inversion. The weighted ensemble means and variances from the hierarchical approach are quite similar to the conventional values because the best model in the ensemble is also quite close to the ensemble mean. The approach can also be used for cross-validation in which some data are held back to test estimates obtained with the rest. We demonstrate this with a test of the TransCom inversions holding back the airborne data. We see a slight decrease in the tropical sink and a notably different preferred order of models.
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    Greenhouse Gas Concentration and Volcanic Eruptions Controlled the Variability of Terrestrial Carbon Uptake Over the Last Millennium
    Zhang, X ; Peng, S ; Ciais, P ; Wang, Y-P ; Silver, JD ; Piao, S ; Rayner, PJ (AMER GEOPHYSICAL UNION, 2019-06)
    The terrestrial net biome production (NBP) is considered as one of the major drivers of interannual variation in atmospheric CO2 levels. However, the determinants of variability in NBP under the background climate (i.e., preindustrial conditions) remain poorly understood, especially on decadal-to-centennial timescales. We analyzed 1,000-year simulations spanning 850-1,849 from the Community Earth System Model (CESM) and found that the variability in NBP and heterotrophic respiration (RH) were largely driven by fluctuations in the net primary production (NPP) and carbon turnover rates in response to climate variability. On interannual to multidecadal timescales, variability in NBP was dominated by variation in NPP, while variability in RH was driven by variation in turnover rates. However, on centennial timescales (100-1,000 years), the RH variability became more tightly coupled to that of NPP. The NBP variability on centennial timescales was low, due to the near cancellation of NPP and NPP-driven RH changes arising from climate internal variability and external forcings: preindustrial greenhouse gases, volcanic eruptions, land use changes, orbital change, and solar activity. Factorial experiments showed that globally on centennial timescales, the forcing of changes in greenhouse gas concentrations were the largest contributor (51%) to variations in both NPP and RH, followed by volcanic eruptions impacting NPP (25%) and RH (31%). Our analysis of the carbon-cycle suggests that geoengineering solutions by injection of stratospheric aerosols might be ineffective on longer timescales.
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    Correction: Causal knowledge promotes behavioral self-regulation: An example using climate change dynamics.
    Sewell, DK ; Rayner, PJ ; Shank, DB ; Guy, S ; Lilburn, SD ; Saber, S ; Kashima, Y (Public Library of Science (PLoS), 2020)
    [This corrects the article DOI: 10.1371/journal.pone.0184480.].
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    Causal knowledge promotes behavioral self-regulation: An example using climate change dynamics
    Sewell, DK ; Rayner, PJ ; Shank, DB ; Guy, S ; Lilburn, SD ; Saber, S ; Kashima, Y ; Perales, JC (PUBLIC LIBRARY SCIENCE, 2017-09-07)
    Adopting successful climate change mitigation policies requires the public to choose how to balance the sometimes competing goals of managing CO2 emissions and achieving economic growth. It follows that collective action on climate change depends on members of the public to be knowledgeable of the causes and economic ramifications of climate change. The existing literature, however, shows that people often struggle to correctly reason about the fundamental accumulation dynamics that drive climate change. Previous research has focused on using analogy to improve people's reasoning about accumulation, which has been met with some success. However, these existing studies have neglected the role economic factors might play in shaping people's decisions in relation to climate change. Here, we introduce a novel iterated decision task in which people attempt to achieve a specific economic goal by interacting with a causal dynamic system in which human economic activities, CO2 emissions, and warming are all causally interrelated. We show that when the causal links between these factors are highlighted, people's ability to achieve the economic goal of the task is enhanced in a way that approaches optimal responding, and avoids dangerous levels of warming.