School of Physics - Theses
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ItemQuasar Broad Emission Line Regions and Gravitational Microlensing( 2023-08)This thesis has focussed on hydrogen and helium emission line generation in the Broad Emission Line Region (BELR) of quasars and also on the gravitationally lensed quasar LBQS1009-0252. Quasars are a class of galaxy characterised by an active nuclear region in which a high rate of accretion onto a central supermassive black hole results in the release of vast amounts of broadband energy over a prolonged period of time. These incredible luminosities—often up to 100,000 times that of a standard galaxy—make quasars some of the most distant, and therefore earliest, sources ever observed in the universe. The relatively tiny size of the innermost region, however, precludes direct observation, and so the physics and geometry of quasars remains enigmatic. Emitted by the accretion disk, light interacts with surrounding gasses in the BELR—so-named because light which is reprocessed and re-emitted from this region tends to be significantly broadened due to wholescale Doppler motions of the gas. As the first gas to ‘see’ light from the accretion disk, understanding and constraining the nature and dynamics of the BELR remains of interest in many astrophysical fields. Following methods pioneered by Ruff (2012), microphysical simulations (such as those produced by the photoionisation code, Cloudy) can be combined with observed spectral data of real sources to model hydrogen line emission from the BELR. This research has confirmed and built further upon the methods presented in Ruff (2012) through the use of updated code and new, high-quality NIR spectral data of 14 quasar sources acquired from the Flamingos-2 (F2) instrument on Gemini South at the Gemini Observatory. The thesis has also gone a step beyond the original method and includes the modelling and analysis of helium emission lines for the first time. Broadly, the results lend support to the conclusions presented in Ruff (2012): hydrogen lines tend to be produced optimally in regions of low incident ionising flux and high gas number density. Helium lines also appear to follow this trend, clustering in a similar parameter space, although there appears to be a tendency towards a flatter distribution across the value for maximum gas number density. This suggests that despite similarities in their physical production and spectral appearance, there are some slight differences in the behaviour of hydrogen and helium emission lines in the BELR, and it is prudent to analyse them separately where possible. This thesis also examined the double-image gravitationally lensed quasar, LBQS1009-0252, via new and relatively high-resolution data from the Gemini Multi-Object Spectrograph (GMOS) at Gemini Observatory. The project investigated both the emission and absorption lines present in the spectra of components A and B, seeking to better understand the spectral differences apparent between the two images. The analysis confirms that the LBQS1009-0252 system likely consists of two images of the same, gravitationally lensed background quasar source, with a third component, LBQS1009-0252C, most likely a foreground and physically unrelated quasar. A comparison and analysis of the overall spectra and emission lines attempts to separate the effects of different light paths through the lensing galaxy, previously identified at z~0.869. A combination of differential extinction due to dust in the macrolens plus a minor component of microlensing is a reasonable explanation for the origin of chromaticity between the spectra of the two component images. The new dataset was of high resolution, allowing for the identification of many more absorption lines than had previously been catalogued. These have been matched to those previously classified as belonging to the lensing galaxy and another known absorber situated at z~1.627. Newly-observed lines were analysed to identify likely absorption species candidates, showing that the presence of at least one more intervening absorption system at z~1.116–1.117 is highly likely.
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ItemMechanisms of ergodicity breaking - from time crystals to Hilbert space fragmentation( 2023-11)The concept of ergodicity reaches back to Boltzmann’s attempts at formalizing and clarifying the foundations of statistical mechanics. The postulate of thermal equilibrium seems to describe the behavior of sufficiently complex real-world systems, whether they are classical or quantum, exceedingly well. However, our understanding of the fundamental laws of physics that govern the dynamics of these systems on a microscopic scale can at first glance seem incompatible with this postulate. A complete description of the dynamical process of thermalization is subject of ongoing research even more than a century after Boltzmann’s contribution. Significant advances have been made, including a formal description of this process in the context of closed quantum systems that is linked to properties of its energy eigenstates. Besides deepening our understanding of what seems to be quite generic behavior, the possibility of robust exceptions to the fundamental postulates of thermodynamics have been unveiled as a consequence. Among them are potentially novel phases of matter, such as many-body localization, time crystals and Hilbert space fragmentation, that do not readily fit within the usual frameworks of phase transitions and may even find application in quantum technologies. In this thesis, I discuss the current state of research in regards to thermalization in quantum systems and some of the presumable exceptions. I then present my own contribution to the field in the form of published works on time crystals and fragmentation. In particular, I demonstrate the realization of a discrete time crystal on a quantum computer, a rapidly evolving technology at the forefront of quantum information science that promises to revolutionize our ability to model and simulate quantum systems. The demonstration of a novel phase of matter in the form of a time crystal represents one of the first successful applications of a quantum device in the field of quantum many-body physics. Furthermore, I present results on interaction-induced fragmentation that address questions about the relationship between localization and fragmentation. They also demonstrate possible transitions between different dynamical regimes within a fragmented system based on tunable emergent conserved charges. Lastly, I present work on the robustness of Hilbert space fragmentation under more general perturbations than are typically considered in other works. Introducing a new definition of block inverse participation ratio, I show that fragmentation may constitute a finite regime within the space of Hamiltonians with a possible phase transition into ergodic dynamics, with the block inverse participation ratio serving as the order parameter.
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ItemTopological quantum computing with magnet-superconductor hybrid systems( 2023-11)Developing a practical general purpose quantum computer is this eras moonshot project, enabling fundamental advances in simulating quantum many-body systems, as well as promising new classical-computer-beating algorithms with applications in cryptography, meteorology, economics, and logistics. Current quantum processors struggle with short coherence times --- meaning that the fragile quantum bits (qubits) break down --- resulting in high error rates. Thus complicated or long calculations are prohibitive to run on current devices. Quantum error correction could be the solution, however, many physical qubits are required to encode a single logical qubit. Thus a massive scaling up of hardware is required to realise even a modest number of fault-tolerant logical qubits. Over the past twenty years the idea of engineering an inherently fault-tolerant, or topological, quantum computer has been developed. In principle, these fault-tolerant qubits do not decohere due to a topological protection; the information is distributed across a physical system such that local perturbations do not damage the whole information encoding. Majorana zero-modes, characteristic quasiparticles in topological superconductors, have emerged as a leading candidate for the building blocks of a fault-tolerant qubit. Many experimental platforms which might yield Majorana zero-modes have been proposed, but as of writing unambiguous evidence for Majorana zero-modes and topological superconductivity has not been presented in any experiment. Here I study magnet-superconductor hybrid (MSH) systems, which involve networks of magnetic adatoms assembled on a superconducting surface via lateral atom manipulation using a scanning tunneling microscope tip. These systems are clean and crystalline, and thus are an ideal platform for experiments. I present compelling theoretical and experimental evidence for topological superconductivity in Mn and Fe chains on Nb(110). However, the systems investigated so far experimentally have long localisation lengths, resulting in hybridised Majorana modes. Because these modes cannot be used to build a fault-tolerant qubit, I theoretically investigate several extensions to these experiments. I propose constructing quasi one-dimensional chains consisting of several rows of magnetic adatoms, with ferromagnetic order in one crystalline direction and antiferromagnetic in the other. I also suggest engineering the Nb(110) surface with an alloy to dramatically increase the Rashba splitting. Both of these proposals are readily accessible in experiment, and could yield non-hybridised Majorana zero-modes. Having established the viability of the platform, I introduce a numerical apparatus for studying many-body nonequilibrium superconducting physics. While this is generic and can be applied to any superconducting problem, here I use it to study topological quantum computing on a MSH platform. I first show that quantum gates can indeed be implemented via braiding Majorana zero-modes. I then show how single-molecule magnets can be use to initialise and readout MSH qubits. I build on this protocol and introduced a dressed Majorana qubit, which combines an MSH network with single-molecule magnets. These could be easier to initialise and readout than a conventional Majorana qubit.
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ItemAddressing domain shift in deeply-learned jet tagging at the LHC( 2023-09)Over the last fifteen years, deep learning has emerged as an extremely powerful tool for exploiting large datasets. At the Large Hadron Collider, which has been in operation over the same time span, an important use case is to identify the initiating particles of hadronic jets. Due to the complexity of the radiation patterns within jets, neural network-based classifiers are able to out-perform traditional techniques for jet tagging. While these approaches are powerful, neural networks must be applied carefully to avoid performance losses in the presence of domain shift—where the data on which a model is evaluated follows different statistics to the training dataset. This thesis presents studies of possible strategies to mitigate domain shift in the application of deep learning to jet tagging. Firstly, we develop a deep generative model that can separately learn the distribution of quark and gluon jets from mixed samples. Building on the jet topics framework, this model provides the ability to sample quark and gluon jets in high dimension without taking input from Monte Carlo simulations. We demonstrate the advantage of the model over a conventional approach in terms of estimating the performance of a quark/gluon classifier on experimental data. One can also use likelihoods under the model to perform classification that is robust to outliers. We go on to evaluate fully- and weakly-supervised classifiers using real datasets collected at the CMS experiment. Two measurements of the quark/gluon mixture proportions of the datasets are made under different assumptions. Compared to the predictions based on simulation, we either over- or under-estimate the quark fractions of each sample depending on which assumption is made. When estimating the discrimination power of the classifiers in real data we find that while the absolute performance depends on the choice of fractions, the rankings among the models are stable. In particular, weakly-supervised models trained on real jets outperform both simulation-trained models. Our generative networks yield competitive classification and provide a better model for the quark and gluon jet topic distributions in data than the simulation. Finally, we investigate the performance of a number of methods for training mass-generalised jet taggers, with a focus on algorithms that leverage meta-learning. We study the discrimination of jets from boosted Z' bosons against a QCD background and evaluate the networks' performance at masses distant from those used in training. We find that a simple data augmentation strategy that standardises the angular scale of jets with different masses is sufficient to produce strong generalisation. The meta-learning algorithms provide only a small improvement in generalisation when combined with this augmentation.
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ItemFunctional Renormalization Group Methods for Spin-Orbit Coupled Hubbard Systems( 2023-08)This thesis establishes the extension of the functional renormalization group to systems of arbitrary lattice complexity with additional spin or orbital degrees of freedom. Using these capabilities, we investigate the effects of spin-orbit coupling on square and triangular lattice structures, which describe for example cuprates, iron-pnictides, strontium ruthenate, tin layers on silicon and lead layers on silicon-carbide. For the methodological advances, we build on previous studies of the truncated-unity functional renormalization group, but remedy existing symmetry breaking issues. These were incurred when combining a sublattice degree of freedom with the expansion of non- transfer momentum dependencies in a plane-wave basis, and can be alleviated by careful selection of considered bonds. We furthermore demonstrate a wide range of intricacies, paramount for correct functional renormalization calculations, all of which we resolved. The obtained algorithms we validate at certainty not hitherto achieved, heralding a novel approach of quantitative comparison. All of this is contained and published in a high- performance C++ implementation, already in use by junior researchers. Motivated by experimental results, we study the effect of Rashba spin-orbit coupling in the square-lattice Hubbard model. We find the superconducting instabilities to be robust under weak-to-moderate Rashba-coupling strengths. When the coupling is increased further the transition scale decreases significantly. We furthermore measure the contribution of triplet superconductivity, to indicate regions of interest for topological effects. Taking advantage of the functional renormalization group’s capability to produce phase diagrams, we also investigate particle-hole instabilities in the system. Here we find a complex interplay of commensurate and incommensurate spin-density waves and unexpected regions of accidental nesting. The weak-to-intermediate coupling phase diagram in filling and spin-orbit coupling strength is presented. We lastly turn our attention to triangular lattice materials. Here, recent ab-initio calculations predict high Rashba spin-orbit coupling strengths in, for example, Pb on SiC. We introduce Rashba spin-orbit coupling to the Hubbard model, finding a wide range of spin-density waves with differing ordering vectors, some of which appear favorable for multi-q instabilities. We further find superconducting phases around half-filling and at low filling. The region around half-filling is singlet-dominated, gaining triplet weight with increased spin-orbit coupling. Contrarily the pure triplet region at low filling is an extended phase, persisting under spin-orbit coupling. We present a phase diagram for the triangular lattice Rashba-Hubbard model in filling and spin-orbit coupling strength.
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ItemMassive Black Holes( 2023-08)Black holes are one of the most fundamental astrophysical objects in our universe. In this thesis I look at massive black holes (MBH) with masses $10^{4}-10^{10}$ times that of our sun. In particular, I investigate how their gravitational influence distorts photon trajectories and describe how this can be used to study MBH. This phenomena, known as gravitational lensing, results in changes in shape and brightness of the images of the source as seen by a distant observer. The most striking manifestation of gravitational lensing is multiple images, known as \emph{strong} gravitational lensing. Strong gravitational lensing also results in the magnification of one or more of the images above that which would have been observed in the absence of deflecting matter. The number of cosmological black holes (MBH that do not belong to a galaxy core) is not well constrained. Gravitational lens statistics is one of the few ways to probe their number density. The fraction of sources experiencing strong gravitational lensing (multiple-image formation) is proportional to the number density of gravitational lenses which are able to form such images. GRBs are short bursts of $\gamma$-rays which signify the birth of a stellar mass black hole. Gravitational lensing of time-series data (light-curves) manifests as repetition of the primary signal as a lensed ``echo''. I describe the Bayesian parameter estimation and model selection software \pygrb{} which I wrote for this thesis. I use \pygrb{} to analyse GRB lens candidates from the Burst And Transient Source Experiment (BATSE) GRB catalogue to determine how similar the putative GRB lensed echo images are. I find one convincing candidate -- GRB~950830 -- which passes all our tests for statistical self-similarity. I conclude that GRB~950830 was gravitationally lensed by a $(1+z_l)M_l\approx\unit[5.5\times 10^4]{\msun}$ intermediate mass black hole (IMBH). Furthermore, based on the occurrence rate of this lensing event, I am able to estimate that the density of IMBH in the universe is $n_\textsc{imbh}=\unit[6.7^{+14.0}_{-4.8}\times10^{3}]{Mpc^{-3}}$. I also study the merger of black holes, looking at the recoiling quasar E1821+643 (E1821 hereafter). E1821 has a mass of $\mbh \sim \unit[2.6\times10^9]{\msun}$ and is moving with a line-of-sight velocity $v_\text{los}\approx \unit[2,070\pm50]{\kms}$ relative to its host galaxy. I use Bayesian inference to infer that E1821+643 was likely formed from a binary black hole system with masses of $m_1\sim 1.9^{+0.5}_{-0.4}\times \unit[10^9]{M_\odot}$, $m_2\sim 8.1^{+3.9}_{-3.2} \times \unit[10^8]{M_\odot}$ (90\% credible intervals). Given our model, the black holes in this binary were likely to be spinning rapidly with dimensionless spin magnitudes of ${\chi}_1 = 0.87^{+0.11}_{-0.26}$, ${\chi}_2 = 0.77^{+0.19}_{-0.37}$. I find that E1821+643 is likely to be rapidly rotating with dimensionless spin ${\chi} = 0.92\pm0.04$. Recoiling black holes are one method to populate the universe with massive black holes, however, these are expected to be rare. Massive black holes carry with them a tight cluster of stars and stellar remnants. These stars will pass through the optical caustic(s) of the black hole occasionally, which may lead to observable brightening of the star. Magnifications of greater than one million can easily be achieved, which I term ``Gargantuan Magnification Events'' (GMEs). I estimate the rate at which this lensing occurs, including the distribution of magnifications and event durations. I consider GMEs of pulsars in orbit of MBH as a possible generating mechanism for Fast Radio Bursts (FRBs). I find that pulsar GMEs are able to account for $0.1-1\%$ of the total FRB rate as observed by the Canadian Hydrogen Intensity Mapping Experiment Fast Radio Burst (CHIME/FRB) radio observatory. These seemingly unrelated problems all tied together in the end. This thesis is a study of black holes, their interaction with light and matter, and how they evolve through cosmic time. Many lifetimes of work have gone into generating the theory behind the sentence just prior. I hope that my contributions embellish these theories.
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ItemDeveloping and applying quantum sensors based on optically addressable spin defects( 2023-04)Quantum sensing aims to further our understanding of the natural world and support an upcoming technological revolution by exploiting quantum properties or systems to exceed the performance of classical sensing. Owing to their convenient modes of operation and strong room temperature quantum properties, optically active spin defects hosted within solid state materials have come to prominence as one of the foremost tools of choice in this landscape. Many applications now aim to leverage dense ensembles of such defects to boost measurement sensitivity or scale up, which places greater emphasis on the quality of the host material and sensor production methods since cherry-picking individual defects is no longer an option. The prototypical example of such a defect is the nitrogen-vacancy (NV) centre in diamond, which exhibits remarkable room temperature spin coherence, bestowed upon it by diamond's material properties. In this thesis, we first look at optimising the production of NV ensembles for quantum sensing, aiming to efficiently and cost-effectively produce sensors capable of performing high sensitivity measurements in two key regimes that will be central to the experimental applications explored later. The topics examined are hyperpolarisation of a nuclear spin ensemble on the diamond surface through coupling to an ultra-near-surface NV layer, and investigating the properties of a van der Waals antiferromagnet through widefield NV microscopy. The demands placed on the NV layer for these applications are diverse from one another, with charge stability and quantum coherence properties being vital for the former, and the ability to scalably and reproducibly create layers of known thickness crucial to the latter. In light of these studies, we finally consider whether a different spin system housed within an entirely separate materials system, the boron-vacancy defect in hexagonal boron nitride, may be a suitable alternative to the well-established NV diamond system. We find that the distinct properties of the new host material provide both advantages and disadvantages compared to diamond, and that this system could allow quantum sensing to find even broader scope in the future. By investigating the link between host material properties and the suitability of a quantum sensor for given applications, this thesis provides a unique perspective on the future of the field, which will likely demand more highly specialised and varied sensors.
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ItemNo Preview AvailableDeterministic implantation of donor ions in near-surface nanoarrays for silicon quantum computing( 2023-08)Remarkable theoretical and experimental progress has been achieved with donor-based silicon quantum computing architectures in the last decade, firmly cementing this implementation as one of the forerunners in the race to build the first large-scale quantum computer. By employing near-surface donor atoms (P, As, Sb, Bi) as the storage medium, both their nuclear and electronic spin states can be used to encode quantum information. Silicon is an excellent host material, having the advantage that donor atoms can easily be incorporated into its lattice, as well as being able to be isotopically enriched into 28Si, giving donor spin coherence times in excess of 30 s. Despite a significant number of experimental challenges, the end goal of creating a near-surface entangled donor array to enable multi-qubit operations is in sight. The aim of this work is to address some significant recent advances towards this goal through the use of directed implantation of single donor ions. Ion implantation has previously been shown to be a valid method for introducing donor-qubits into silicon, and for decades has been a well-established fabrication technique in the classical semiconductor industry. In this work, it is shown that by employing silicon-based active detection substrates connected to an ultra-low noise charge-sensitive preamplifier, single donor ions can be deterministically implanted at depths between 10 - 20 nm with a detection confidence exceeding 99.8%. The recent acquisition of an in-situ stepped nanostencil extends this concept further to allow the controlled placement of single donors to a lateral precision of around 50 nm. Through the use of a step-and-repeat procedure, the ability to form two-dimensional qubit nanoarrays with this system is demonstrated. With the technique readily capable of scaling up to hundreds of qubits or more, this represents a significant milestone towards the realisation of a top-down solid state qubit architecture. A complementary method for single donor placement in silicon is also given, again using ion implantation. It involves the use of a focused ion beam instrument that has been modified to include a keV electron-beam-ion-source to give access to a large selection of ion species, focused to a 180 nm spot size. By integration of the same high-confidence single ion detection technology, it is shown that this technique is also capable of creating large-scale donor arrays in silicon, but without the need for a physical mask. Its use as not just a single ion implanter, but also a novel instrument for near-surface characterisation of semiconductors is also presented. The system's functionality is demonstrated through the identification of fabrication faults in a silicon-based device that otherwise may have gone undetected through conventional characterisation methods. The adaptation of the focused ion beam technique into an efficient method for creating micro-volumes of isotopically pure 28Si is also explored. This is an important area of focus required to achieve ultra-long qubit coherence times, with the results of a preliminary characterisation confirming the technique's suitability. Finally, adapting the single ion detection technology to demonstrate a new approach for performing high-resolution Rutherford backscattering spectrometry is also presented. Some major advantages include a small physical detector footprint and ease of integration into existing beamline structures. In keeping with the overall theme of this study, the system is used to analyse samples pertinent to silicon donor quantum computing, such as shallowly implanted donors and enriched 28Si wafers. The series of experiments performed in this thesis thus represent some significant steps towards achieving the scalable fabrication of a donor-based silicon quantum computer.
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ItemTowards Automating the Design and Optimisation of Particle Accelerators( 2023-06)The question of efficiency and optimality of accelerator lattice structures was investigated in this thesis. Within the context of circular accelerators for hadron therapy, an analysis on the design methodology of existing compact circular acceler-ators was carried out. This analysis prompted the design of a novel lattice based on two double bend achromat arcs as an alternative to conventional periodic cell struc-tures. The feasibility to perform slow extraction for hadron therapy purposes was demonstrated using the proposed lattice. The extraction efficiency was optimised by tuning the lattice optics. In the second half of this thesis, an automated design and optimisation algorithm was proposed. This algorithm was developed as a general purpose lattice design tool. The development process examined three optimisation routines including the Simulated Annealing algorithm, a simple genetic algorithm, and the Non-dominated Sorting Genetic Algorithm (NSGA). Three encoding methods were developed to represent the accelerator lattice for use with the optimisation routines. Namely, the finite slicing encoder, the neural network encoder, and the matrix encoder. It was found that the combination of NSGA-III algorithm and the matrix encoder was the most efficient method for exploring the feasible parameter space for a generalisable lattice design problem.
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ItemSurface acoustic wave neuromodulation( 2023-03)Neurological disorders such as Alzheimer's disease often involve impaired axonal function, underscoring the importance of modulating diffusion processes within axons for treatment. Surface Acoustic Waves (SAWs) offer a promising avenue for this, given their unique properties like miniaturized dimensions, absence of shock waves, and reduced self-heating compared to traditional ultrasound methods. This thesis explores the utility of SAWs in enhancing axonal diffusion as a potential treatment for neurological disorders characterized by axonal dysfunction. The initial phase of the research employed retinal ganglion cells as a model system for studying diffusion. The axons of retinal ganglion cells are naturally radially aligned and serve as a well-established model, offering advantages in data analysis and reducing error. A mathematical model was established to measure dye diffusion in these cells, laying the groundwork for understanding diffusion mechanisms that are broadly applicable, including but not limited to Alzheimer's disease. Subsequently, I investigated the SAW-driven diffusion enhancement in artificial axons, represented by microchannels. My findings indicate up to a 39% increase in diffusion rates within these microchannels when subjected to SAWs. Numerical simulations were conducted to understand the acoustic pressure fields and acoustic streaming fields, elucidating the mechanisms behind SAW-based diffusion enhancement. Lastly, I explored the biological implications of SAWs by studying their effects on astrocyte recovery, a key factor in brain injury treatment. My results demonstrate that SAWs can promote astrocyte coverage and extrusion growth without affecting width, primarily through enhanced cellular activity rather than increased membrane permeability. Overall, this thesis contributes a new analytical approach to measuring diffusion, advances our understanding of SAW-based mechanisms, and offers a novel potential treatment avenue for neurological disorders involving axonal dysfunction.