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    X-ray diffractive imaging of controlled gas-phase molecules: Toward imaging of dynamics in the molecular frame

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    Author
    Kierspel, T; Morgan, A; Wiese, J; Mullins, T; Aquila, A; Barty, A; Bean, R; Boll, R; Boutet, S; Bucksbaum, P; ...
    Date
    2020-02-28
    Source Title
    Journal of Chemical Physics
    Publisher
    AMER INST PHYSICS
    University of Melbourne Author/s
    Morgan, Andrew
    Affiliation
    School of Physics
    Metadata
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    Document Type
    Journal Article
    Citations
    Kierspel, T., Morgan, A., Wiese, J., Mullins, T., Aquila, A., Barty, A., Bean, R., Boll, R., Boutet, S., Bucksbaum, P., Chapman, H. N., Christensen, L., Fry, A., Hunter, M., Koglin, J. E., Liang, M., Mariani, V., Natan, A., Robinson, J. ,... Kuepper, J. (2020). X-ray diffractive imaging of controlled gas-phase molecules: Toward imaging of dynamics in the molecular frame. JOURNAL OF CHEMICAL PHYSICS, 152 (8), https://doi.org/10.1063/1.5133963.
    Access Status
    Access this item via the Open Access location
    URI
    http://hdl.handle.net/11343/254045
    DOI
    10.1063/1.5133963
    Open Access URL
    https://bib-pubdb1.desy.de/record/436490/files/1.5133963.pdf
    Abstract
    We report experimental results on the diffractive imaging of three-dimensionally aligned 2,5-diiodothiophene molecules. The molecules were aligned by chirped near-infrared laser pulses, and their structure was probed at a photon energy of 9.5 keV (λ ≈ 130 pm) provided by the Linac Coherent Light Source. Diffracted photons were recorded on the Cornell-SLAC pixel array detector, and a two-dimensional diffraction pattern of the equilibrium structure of 2,5-diiodothiophene was recorded. The retrieved distance between the two iodine atoms agrees with the quantum-chemically calculated molecular structure to be within 5%. The experimental approach allows for the imaging of intrinsic molecular dynamics in the molecular frame, albeit this requires more experimental data, which should be readily available at upcoming high-repetition-rate facilities.

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