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dc.contributor.authorKierspel, T
dc.contributor.authorMorgan, A
dc.contributor.authorWiese, J
dc.contributor.authorMullins, T
dc.contributor.authorAquila, A
dc.contributor.authorBarty, A
dc.contributor.authorBean, R
dc.contributor.authorBoll, R
dc.contributor.authorBoutet, S
dc.contributor.authorBucksbaum, P
dc.contributor.authorChapman, HN
dc.contributor.authorChristensen, L
dc.contributor.authorFry, A
dc.contributor.authorHunter, M
dc.contributor.authorKoglin, JE
dc.contributor.authorLiang, M
dc.contributor.authorMariani, V
dc.contributor.authorNatan, A
dc.contributor.authorRobinson, J
dc.contributor.authorRolles, D
dc.contributor.authorRudenko, A
dc.contributor.authorSchnorr, K
dc.contributor.authorStapelfeldt, H
dc.contributor.authorStern, S
dc.contributor.authorThogersen, J
dc.contributor.authorYoon, CH
dc.contributor.authorWang, F
dc.contributor.authorKuepper, J
dc.date.accessioned2020-12-14T05:54:53Z
dc.date.available2020-12-14T05:54:53Z
dc.date.issued2020-02-28
dc.identifier.citationKierspel, T., Morgan, A., Wiese, J., Mullins, T., Aquila, A., Barty, A., Bean, R., Boll, R., Boutet, S., Bucksbaum, P., Chapman, H. N., Christensen, L., Fry, A., Hunter, M., Koglin, J. E., Liang, M., Mariani, V., Natan, A., Robinson, J. ,... Kuepper, J. (2020). X-ray diffractive imaging of controlled gas-phase molecules: Toward imaging of dynamics in the molecular frame. JOURNAL OF CHEMICAL PHYSICS, 152 (8), https://doi.org/10.1063/1.5133963.
dc.identifier.issn0021-9606
dc.identifier.urihttp://hdl.handle.net/11343/254045
dc.description.abstractWe report experimental results on the diffractive imaging of three-dimensionally aligned 2,5-diiodothiophene molecules. The molecules were aligned by chirped near-infrared laser pulses, and their structure was probed at a photon energy of 9.5 keV (λ ≈ 130 pm) provided by the Linac Coherent Light Source. Diffracted photons were recorded on the Cornell-SLAC pixel array detector, and a two-dimensional diffraction pattern of the equilibrium structure of 2,5-diiodothiophene was recorded. The retrieved distance between the two iodine atoms agrees with the quantum-chemically calculated molecular structure to be within 5%. The experimental approach allows for the imaging of intrinsic molecular dynamics in the molecular frame, albeit this requires more experimental data, which should be readily available at upcoming high-repetition-rate facilities.
dc.languageEnglish
dc.publisherAMER INST PHYSICS
dc.titleX-ray diffractive imaging of controlled gas-phase molecules: Toward imaging of dynamics in the molecular frame
dc.typeJournal Article
dc.identifier.doi10.1063/1.5133963
melbourne.affiliation.departmentSchool of Physics
melbourne.source.titleJournal of Chemical Physics
melbourne.source.volume152
melbourne.source.issue8
melbourne.elementsid1441280
melbourne.openaccess.urlhttps://bib-pubdb1.desy.de/record/436490/files/1.5133963.pdf
melbourne.openaccess.statusPublished version
melbourne.contributor.authorMorgan, Andrew
dc.identifier.eissn1089-7690
melbourne.accessrightsAccess this item via the Open Access location


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